Keywords
Electroactive materials
Organic electrode materials
Organic batteries
Lithium batteries
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Abstract
Electroactive organic materials have attracted considerable interest as alternative elec-trodes for metal-ion batteries due to their high theoretical capacity, resource availability, and sustainability. In particular, redox-active covalent organic frameworks (COFs) have recently emerged as promising electrodes owing to their tunable electrochemical proper-ties, insolubility in electrolytes, and high structural versatility. This article reviews recent strategies for improving the energy density of COF-based electrodes from the perspective of molecular design and electrode optimization. Other relevant aspects, such as stability and scalability, are also discussed. Finally, the main challenges to further enhance their performance and the future prospects of COF-based organic batteries are highlighted.
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